Statistical clumped isotope signatures

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Statistical clumped isotope signatures

High precision measurements of molecules containing more than one heavy isotope may provide novel constraints on element cycles in nature. These so-called clumped isotope signatures are reported relative to the random (stochastic) distribution of heavy isotopes over all available isotopocules of a molecule, which is the conventional reference. When multiple indistinguishable atoms of the same e...

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Methane cold seep systems typically exhibit extensive buildups of authigenic carbonate minerals, resulting from local increases in alkalinity driven by methane oxidation. Here, we demonstrate that modern seep authigenic carbonates exhibit anomalously low clumped isotope values (Δ47), as much as ∼0.2‰ lower than expected values. In modern seeps, this range of disequilibrium translates into appar...

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A revised calibration of the clumped isotope thermometer

Article history: Received 5 December 2012 Received in revised form 3 July 2013 Accepted 16 July 2013 Available online xxxx Editor: G. Henderson

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Antarctic ice growth before and after the Eocene-Oligocene transition: New estimates from clumped isotope paleothermometry

Across the Eocene-Oligocene transition, the oxygen isotopic composition (δO) of benthic and planktonic foraminifera increased by over 1‰. This shift is thought to represent a combination of global cooling and the growth of a large ice sheet on the Antarctic continent. To determine the contribution of each of these factors to the total change in δO, we measured the clumped isotopic composition o...

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ژورنال

عنوان ژورنال: Scientific Reports

سال: 2016

ISSN: 2045-2322

DOI: 10.1038/srep31947